this is all theoretical, but this is what i would try...
i think if you open your iphone's settings in iTunes, and open the "info" tab at the top, you can set it to sync your contacts to the mac's address book. As of now, it's probably set to entourage or Exchange or whatever...
so i think if you switch it to the Mac's address Book for one sync, and choose to "merge contacts" between your phone and Mac, then it will do it. Once that is complete, switch the setting in iTunes back to sync with entourage or exchange, and then it will resume syncing with your exchange server, but your mac will remember the contacts that were synced to it.
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