After my iPhone is synced to the computer, I uncheck the music/videos I want to remove and apply the changes. Once off the iPhone, I go into the library section of iTunes and delete the file from the iTunes library. Note, the original copy of the file I'm deleting remains untouched in my external drive.
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-Larry and Harry Spotter
We're on the iRovr EIC stream
16 GB iPhone 3G 
8 GB iPhone 2G
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